分类： 光学 >> 量子光学 提交时间： 2023-02-19
摘要： The key component of nanoplasmonics is metals. For a long time, gold and silver have been the metals of choice for constructing plasmonic nanodevices because of their excellent optical properties. However, these metals possess a common characteristic, i.e., their optical responses are static. The past decade has been witnessed tremendous interest in dynamic control of the optical properties of plasmonic nanostructures. To enable dynamic functionality, several approaches have been proposed and implemented. For instance, plasmonic nanostructures can be fabricated on stretchable substrates or on programmable templates so that the interactions between the constituent metal nanoparticles and therefore the optical responses of the plasmonic systems can be dynamically changed. Also, plasmonic nanostructures can be embedded in tunable dielectric materials, taking advantage of the sensitive dependence of the localized surface plasmon resonances on the neighboring environment. Another approach, which is probably the most intriguing one, is to directly regulate the carrier densities and dielectric functions of the metals themselves.
分类： 光学 >> 量子光学 提交时间： 2023-02-19
摘要： Control over plasmonic colors on the nanoscale is of great interest for high-resolution display, imaging, and information encryption applications. However, so far, very limited schemes have been attempted for dynamic plasmonic color generation. In this paper, we demonstrate a scanning plasmonic color generation scheme, in which subwavelength plasmonic pixels can be laterally switched on/off through directional hydrogenation/dehydrogenation of a magnesium screen. We show several dynamic plasmonic color displays with different scanning functions by varying the number and geometries of the palladium gates, where hydrogen enters the scanning screens. In particular, we employ the scanning effects to create a dynamic plasmonic quick response code. The information cannot be decrypted by varying the polarization states of light or by accessing the physical features. Rather, it can only be read out using hydrogen as a decoding key. Our work advances the established design concepts for plasmonic color printing and provides insights into the development of optical information storage and anticounterfeiting features.
分类： 光学 >> 量子光学 提交时间： 2023-02-19
摘要： One of the fundamental challenges in nanophotonics is to gain full control over nanoscale optical elements. The precise spatiotemporal arrangement determines their interactions and collective behavior. To this end, DNA nanotechnology is employed as an unprecedented tool to create nanophotonic devices with excellent spatial addressability and temporal programmability. However, most of the current DNA-assembled nanophotonic devices can only reconfigure among random or very few defined states. Here, we demonstrate a DNA-assembled rotary plasmonic nanoclock. In this system, a rotor gold nanorod can carry out directional and reversible 360 degree rotation with respect to a stator gold nanorod, transitioning among 16 well-defined configurations powered by DNA fuels. The full-turn rotation process is monitored by optical spectroscopy in real time. We further demonstrate autonomous rotation of the plasmonic nanoclock powered by DNAzyme-RNA interactions. Such assembly approaches pave a viable route towards advanced nanophotonic systems entirely from the bottom-up.
点击量
待评议
点击量
下载量
评论
