分类： 光学 >> 量子光学 提交时间： 2023-02-19
摘要： We propose a composite acousto-optical modulation (AOM) scheme for wide-band, efficient modulation of CW and pulsed lasers. We show that by adjusting the amplitudes and phases of weakly-driven daughter AOMs, diffraction beyond the Bragg condition can be achieved with exceptional efficiencies. Furthermore, by imaging pairs of AOMs in a counter-propagating configuration, high contrast switching of output orders can be achieved at the driving radio frequency (rf) limit, thereby enabling efficient bidirectional routing of a synchronized mode-locked laser. Here we demonstrate a simplest example of such scheme with a double-AOM setup for efficient diffraction across an octave of rf bandwidth, and for routing a mode-locked pulse train with up to $f_{\rm rep}=400$~MHz repetition rate. We discuss extension of the composite scheme toward multi-path routing and time-domain multiplexing, so as to individually shape each pulses of ultrafast lasers for novel quantum control applications.
分类： 光学 >> 量子光学 提交时间： 2023-02-19
摘要： To generate laser with short wavelength is a bottle-neck problem in laser technology. The extreme ultraviolet (EUV) lasers are usually produced with low efficiency by nonlinear multi-photon process. Here we show the generation of 58.4 nm laser by a single-photon-excitation related stimulated anti-Stokes Raman scattering (ASRS) with an efficiency higher than that of high harmonic generation (HHG). Utilizing microwave excited helium in the metastable 1s2s state irradiated by a resonant femto-second 2058 nm laser, we obtain pulsed 58.4 nm laser with a divergence of 1.9 mrad, suggesting its coherent character. The pulse decay time of 426 ps shorter than the lifetime of spontaneous emission also shows its stimulated property. Our results show an applicable path towards up-conversion by single-photon process to generate intense laser with wavelength shorter than 58.4 nm.
分类： 光学 >> 量子光学 提交时间： 2023-02-19
Changqin Liu
Sheng Zhang
Shunjia Wang
Qingnan Cai
Peng Wang
Chuanshan Tian
Lei Zhou
Yizheng Wu
Zhensheng Tao
摘要： The ability to manipulate the electric-field vector of broadband terahertz waves is essential for applications of terahertz technologies in many areas, and can open up new possibilities for nonlinear terahertz spectroscopy and coherent control. Here, we propose a novel laser-driven terahertz emitter, consisting of metasurface-patterned magnetic multilayer heterostructures. Such hybrid terahertz emitters can combine the advantages of spintronic emitters for being ultrabroadband, efficient and flexible, as well as those of metasurfaces for the unique capability to manipulate terahertz waves with high precision and degree of freedom. Taking a stripe-patterned metasurface as an example, we demonstrate the generation of broadband terahertz waves with tunable chirality. Based on experimental and theoretical studies, the interplay between the laser-induced spintronic-origin currents and the metasurface-induced transient charges/currents are investigated, revealing the strong influence on the device functionality originated from both the light-matter interactions in individual metasurface units and the dynamic coupling between them. Our work not only offers a flexible, reliable and cost-effective solution for chiral terahertz wave generation and manipulation, but also opens a new pathway to metasurface-tailored spintronic devices for efficient vector-control of electromagnetic waves in the terahertz regime.
分类： 光学 >> 量子光学 提交时间： 2023-02-23
Bingbing Zhu
Zongyuan Fu
Yudong Chen
Sainan Peng
Cheng Jin
Guangyu Fan
Sheng Zhang
Shunjia Wang
Hao Ru
Chuanshan Tian
Yihua Wang
Henry Kapteyn
Margaret Murnane
Zhensheng Tao
摘要： The high power and variable repetition rate of Yb femtosecond lasers make them very attractive for ultrafast science. However, for capturing sub-200 fs dynamics, efficient, high-fidelity, and high-stability pulse compression techniques are essential. Spectral broadening using an all-solid-state free-space geometry is particularly attractive, as it is simple, robust, and low-cost. However, spatial and temporal losses caused by spatio-spectral inhomogeneities have been a major challenge to date, due to coupled space-time dynamics associated with unguided nonlinear propagation. In this work, we use all-solid-state free-space compressors to demonstrate compression of 170 fs pulses at a wavelength of 1030nm from a Yb:KGW laser to ~9.2 fs, with a highly spatially homogeneous mode. This is achieved by ensuring that the nonlinear beam propagation in periodic layered Kerr media occurs in soliton modes and confining the nonlinear phase through each material layer to less than 1.0 rad. A remarkable spatio-spectral homogeneity of ~0.87 can be realized, which yields a high efficiency of >50% for few-cycle compression. The universality of the method is demonstrated by implementing high-quality pulse compression under a wide range of laser conditions. The high spatiotemporal quality and the exceptional stability of the compressed pulses are further verified by high-harmonic generation. This work represents the highest efficiency and the best spatio-spectral quality ever achieved by an all-solid-state free-space pulse compressor for few-cycle-pulse generation.
分类： 光学 >> 量子光学 提交时间： 2023-02-19
Zongyuan Fu
Yudong Chen
Sainan Peng
Bingbing Zhu
Baochang Li
Rodrigo Martín-Hernández
Guangyu Fan
Yihua Wang
Carlos Hernández-García
Cheng Jin
Margaret Murnane
Henry Kapteyn
Zhensheng Tao
摘要： Extending the photon energy range of bright high-harmonic generation to cover the entire soft X-ray region is important for many applications in science and technology. The concept of critical ionization fraction has been essential, because it dictates the maximum driving laser intensity that can be used while preserving bright harmonic emission. In this work, we reveal a second, nonadiabatic critical ionization fraction that substantially extends the maximum phase-matched high-harmonic photon energy, that arises due to strong reshaping of the intense driving laser field. We validate this understanding through a systematic comparison between experiment and theory, for a wide range of pulse durations and driving laser wavelengths. In particular, high harmonics driven by intense few-cycle pulses experience the most pronounced spectral reshaping, significantly extending the bright photon energy range. We also present an analytical model that predicts the spectral extension that can be achieved for different driving lasers. This reveals an increasing role of nonadiabatic critical phase matching when driven by few-cycle mid-infrared lasers. These findings are important for the development of high-brightness soft X-ray sources for applications in spectroscopy and imaging.
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