分类： 核科学技术 >> 裂变堆工程技术 提交时间： 2023-06-18 合作期刊: 《Nuclear Science and Techniques》
摘要： The Chinese Academy of Science has launched a thorium-based molten-salt reactor (TMSR) research project with a mission to research and develop a fission energy system of the fourth generation. The TMSR project intends to construct a liquid fuel molten-salt reactor (TMSR-LF), which uses fluoride salt as both the fuel and coolant, and a solid fuel molten-salt reactor (TMSR-SF), which uses fluoride salt as coolant and TRISO fuel. An optimized 2 MWth TMSR-LF has been designed to solve major technological challenges in the Th-U fuel cycle. Preliminary conceptual shielding design has also been performed to develop bulk shielding. In this study, the radiation dose and temperature distribution of the shielding bulk due to the core were simulated and analyzed by performing Monte Carlo simulations and computational fluid dynamics (CFD) analysis. The MCNP calculated dose rate and neutron and gamma spectra indicate that the total dose rate due to the core at the external surface of the concrete wall was 1.91 Sv/h in the radial direction, 1.16 Sv/h above and 1.33 Sv/h below the bulk shielding. All the radiation dose rates due to the core were below the design criteria. Thermal analysis results show that the temperature at the outermost surface of the bulk shielding was 333.86 K, which was below the required limit value. The results indicate that the designed bulk shielding satisfies the radiation shielding requirements for the 2 MWth TMSR-LF.
分类： 核科学技术 >> 裂变堆工程技术 提交时间： 2023-06-18 合作期刊: 《Nuclear Science and Techniques》
摘要： The rapid development of nuclear technology has led to more liquid organic radioactive wastes. Different from the regular aqueous radioactive wastes, these liquids possess a higher hazard potential and cannot be disposed through the conventional methods due to their radioactivity and chemical nature. Spent extraction solvent is a kind of common liquid organic radioactive wastes. In this work, tri-butyl phosphate (TBP), which is more difficult to degrade in the spent extraction solvent, was used as the model compound. Influences of reaction conditions on total organic carbon (TOC) removal and the volume percentage of each gas component under supercritical water oxidation (SCWO) were studied. The SCWO behaviors of spent extraction solvent simulants were studied under the optimal conditions derived from the TBP experiment. The SCWO experiments were studied at 400550 ℃, oxidant stoichiometric ratio of 0200%, feed concentration of 1.5%4% and pressure of 25 MPa for 1575 s. The results show that the TOC removal of the simulants was greater than 99.7% and CH4, H2 and CO were not detected at 550 ℃, 25 MPa, oxidant stoichiometric ratio of 150%, feed concentration of 3%, and residence time of 30 s.
分类： 核科学技术 >> 粒子加速器 提交时间： 2023-06-18 合作期刊: 《Nuclear Science and Techniques》
摘要： Photoneutrons, emitted by means of photonuclear interactions when gas bremsstrahlung interacts with beamline components, can be another potential radiation source needed to be considered for shielding design and dose assessment of beamline. In this paper, simulations and measurements of photoneutrons dose rate at beamline BL09U are carried out when Shanghai Synchrotron Radiation Facility (SSRF) running at Top-up mode (3.5 GeV, 235 mA). A geometry model is constructed for the beamline BL09U with considerations of the scattering process of the major optical components. The model is compiled into Monte Carlo simulation code FLUKA to calculate photoneutron dose distribution. Measurements of the photoneutrons dose rate were performed by using Environmental Neutron Monitor (ENM). Observation points were arranged uniformly along the inside and outside of the optical enclosure (OE) of BL09U. The calculation results agree with experiments within the measurements uncertainties. It is verified that photoneutrons dose simulation is reliable. The simulation and measurement methods can be applied to evaluate the neutron dose level of other beamline stations, and provide references for the shielding design of the beamlines at SSRF in the near future.
分类： 核科学技术 >> 裂变堆工程技术 提交时间： 2023-06-18 合作期刊: 《Nuclear Science and Techniques》
摘要： In a molten salt reactor (MSR), the fuel is dissolved in fluoride salt. In this paper, the reactivity worth and reactivity initiated transient of Molten-Salt Reactor Experiment (MSRE) in the control rod failure events are analyzed. The point kinetic coupling heat-transfer model with decay character of six-group delayed neutron precursors due to the fuel motion is applied. The relative power and temperature transient under reactivity step and ramp initiated at different power levels are studied. The results show that the reactor power and temperature increase to a maximum, where they begin to decrease to stable values. Comparing with full power level, the transient result at low power level is more serious. The results are of help in our study on safety characteristics of an MSR system.
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